Factors which Affect and Limit the Performance of Substituted Tris(bipyridine)cobalt(II) Complexes in Dye-sensitized Solar Cells

Factors which Affect and Limit the Performance of Substituted Tris(bipyridine)cobalt(II) Complexes in Dye-sensitized Solar Cells

222 pages· 2007· ISBN 9780549443636
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A suite of DSSC characterization experiments was developed which could be rapidly performed on a standard two electrode sandwich cell. In combination with a novel technique for mediator replacement without cell disassembly, this suite was utilized to probe the influence of several parameters on DSSC functioning in order to identify limitations of cells mediated by cobalt complexes. The results clearly implicate diffusion of cobalt(III) to the cathode as frequently rate-limiting.

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